I think the problem is that Slack is one of those annoying Electron-based apps which is just really a webapp in html/js rendered via an embedded chrome instance. I have tried various combinations of the ControlSend invocation, to no avail.
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ControlSend, Chrome_WidgetWin_1, this is a test, Slack
ControlSend, , this is a test, slack.exe
ControlSend, Chrome_WidgetWin_1, this is a test, slack.exe